改性粉煤灰基烟气脱汞吸附剂氧化性能分析
CSTR:
作者:
作者单位:

作者简介:

通讯作者:

中图分类号:

基金项目:

国家科技支撑计划项目(2007BAC24B03)


Oxidation capability of modified fly ash based adsorbent for mercury in coal-fired flue gas
Author:
Affiliation:

Fund Project:

  • 摘要
  • |
  • 图/表
  • |
  • 访问统计
  • |
  • 参考文献
  • |
  • 相似文献
  • |
  • 引证文献
  • |
  • 资源附件
  • |
  • 文章评论
    摘要:

    为提高粉煤灰基吸附剂对单质汞的氧化性能,分别用NaBr、NaCl溶液对粉煤灰基烟气脱汞吸附剂进行浸渍改性,分析了改性前后吸附剂的物理性能,并研究了改性溶液浓度和烟气温度对Hg 0氧化率的影响。结果表明:用浓度为5%的NaBr溶液改性得到的吸附剂对汞的氧化率为79.43%,饱和吸附量约为1 700 ng/g,使用寿命约为480 h。烟气温度对Hg 0的氧化吸附影响显著,最佳温度范围为100~200 ℃。

    Abstract:

    Fly ash based adsorbent is dipping modified by NaCl or NaBr solution and the purpose is to improve their oxidation capability. Adsorption experiments of vapor-phase elemental mercury are performed in a laboratory-scale fixed-bed reactor. Physical properties of the adsorbent before and after modification are measured and the influences of the solution concentration and flue gas temperature on mercury oxidation rate are studied. The results show that when NaBr solution concentration is 5%, the mercury oxidation rate can reach 79.43%. The saturation adsorption quantity of absorbent 5%-NaBr is 1 700 ng/g and the service life is about 480 hours. Flue gas temperature played an important role in mercury oxidation and the best temperature ranged from 100 to 200 ℃.

    参考文献
    相似文献
    引证文献
引用本文

许志鹏,刘清才,姚春玲,杨剑,卫敏.改性粉煤灰基烟气脱汞吸附剂氧化性能分析[J].重庆大学学报,2012,35(11):81-85.

复制
分享
文章指标
  • 点击次数:
  • 下载次数:
  • HTML阅读次数:
  • 引用次数:
历史
  • 收稿日期:
  • 最后修改日期:
  • 录用日期:
  • 在线发布日期: 2012-12-26
  • 出版日期:
文章二维码